SunnyNet learns the mapping the between LTE and NLTE populations of a model atom and predicts the NLTE populations based on LTE populations for an arbitrary 3D atmosphere. To use SunnyNet, one must already have a set of LTE and NLTE populations computed in 3D, to train the network. These must come from another code, as SunnyNet is unable to solve the formal problem. Once SunnyNet is trained, one can feed it LTE populations from a different 3D atmosphere, and obtain predicted NLTE populations. The NLTE populations can then be used to synthesize any spectral line that is included in the model atom. SunnyNet's output is a file with predicted NLTE populations. SunnyNet itself does not calculate synthetic spectra, but a sample script written in the Julia language that quickly computes Hα spectra is included.